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Fathizadeh, Mahdi ; Tien, Huynh Ngoc ; Khivantsev, Konstantin ; Chen, Jung-Tsai ; Yu, Miao ( , J. Mater. Chem. A)We demonstrated for the first time that inkjet printing can be a low-cost, easy, fast, and scalable method for depositing ultrathin (7.5–60 nm) uniform graphene oxide (GO) nanofiltration membranes on polymeric supports for highly effective water purification. A large area (15 × 15 cm 2 ) GO nanofiltration membrane was printed successfully on a modified polyacrylonitrile (M-PAN) support. Water permeance and rejection of small organic molecules (<1 nm, charged and uncharged) of printed GO membranes can be adjusted by controlling the GO “ink” concentration and/or printing time. Compared with commercial polymeric nanofiltration membranes, printed GO membranes, after optimization, showed approximately one order of magnitude higher water permeance and much higher rejection (>95%) of small organic molecules. Printed GO membranes also showed excellent performance in removing pharmaceutical contaminants, with ∼95% rejection and <10% water permeance decline over extended-period permeation testing. We believe that inkjet printing could be an effective method for preparing ultrathin GO membranes for effective water nanofiltration purification.more » « less
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Khivantsev, Konstantin ; Biancardi, Alessandro ; Fathizadeh, Mahdi ; Almalki, Fahad ; Grant, Job L. ; Tien, Huynh Ngoc ; Shakouri, Abolfazl ; Blom, Douglas A. ; Makris, Thomas M. ; Regalbuto, John R. ; et al ( , ChemCatChem)